While we can’t natively run LibreOffice from within ChromeOS, we can run LibreOffice on a Chromebook using Linux Development Environment. So in this video we demonstrate how from the Linux command prompt, we installed LibreOffice onto our Chromebook.
Notes: In order to run LibreOffice from a Chromebook, you will need to install Linux Development Environment (LDE). LDE is really just a Virtual Machine of Linux within ChromeOS. So by default Linux will be isolated from ChromeOS and any data you have stored on it. If you are using a school or work Chromebook you might not be able to use Linux. So please contact your system administrator or tech support before trying.